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JAEA Reports

Melting temperature of uranium - plutonium mixed oxide fuel

Ishii, Tetsuya; Hirosawa, Takashi

PNC TN9410 97-075, 20 Pages, 1997/08

PNC-TN9410-97-075.pdf:0.71MB

Fuel melting temperature is one of the major thermodynamical properties that is used for determining the design criteria on fuel temperature during irradiation in FBR. In general, it is necessary to evaluate the correlation of fuel melting temperature to confirm that the fuel temperature must be kept below the fuel melting temperature during irradiation at any conditions. The correlations of the melting temperature of uranium-plutonium mixed oxide (MOX) fuel, typical FBR fuel, used to be estimated and formulized based on the measured values reported in 1960's and has been applied to the design. At present, some experiments have been accumulated with improved experimental techniques. And it reveals that the recent measured melting temperatures does not agree well to the data reported in 1960's and that some of the 1960's data should be modified by taking into account of the recent measurements. In this study, the experience of melting temperature up to now are summarized and evaluated in order to make the fuel pin design more reliable. The effect of plutonium content, oxygen to metal ratio and burnup on MOX fuel melting was examined based on the recent data under the UO$$_{2}$$ - PuO$$_{2}$$ - PuO$$_{1.61}$$ ideal solution model, and then formulized. The correlation obtained in this work is as-follows; T = T$$_{0}$$ + $$Delta$$T$$_{Pu}$$ + $$Delta$$T$$_{O/M}$$ + $$Delta$$T$$_{Bu}$$ ----(A) T$$_{0}$$ = 3120 $$Delta$$T$$_{Pu}$$ = -5.7537$$times$$PU + 1.3631$$times$$10$$^{-2}$$ $$times$$ PU$$^{2}$$ + 1.7952$$times$$10$$^{-5}$$ $$times$$ PU$$^{3}$$ $$Delta$$T$$_{O/M}$$ = -1.41 $$times$$ PU $$times$$ (2.00 - OP)/0.39 OP : OP = ${OM - 0.02$times$(100.0 - PU)}$/(0.01$$times$$PU) $$Delta$$T$$_{Bu}$$ = -5.0$$times$$BU/10000 where T is the melting temperature (degree of K), PU is the weight fraction of PuO$$_{2}$$ in the mixed oxide fuel, OM is the oxygen to metal ratio, and BU is the burnup in the unit of MWd/MTM. respectively. $$Delta$$ T$$_{Pu}$$ (plutonium content), $$Delta$$ T$$_{O/M}$$ (O/M Ratio), $$delta$$ ...

JAEA Reports

None

PNC TJ1407 94-001, 56 Pages, 1994/12

PNC-TJ1407-94-001.pdf:4.68MB

no abstracts in English

JAEA Reports

None

; Nemoto, Takeshi; Numata, Koji; *; *; Hanawa, Eiji*; *

PNC TN8440 94-011, 19 Pages, 1994/04

PNC-TN8440-94-011.pdf:0.42MB

None

Journal Articles

Dissolution of plutonium dioxide by electrolytic oxidation method, II; Scaling-up experiments and purification of plutonium

Sakurai, Satoshi; Usuda, Shigekazu; ; Hirata, Masaru; ; Tachimori, Shoichi

Nihon Genshiryoku Gakkai-Shi, 35(2), p.147 - 154, 1993/02

no abstracts in English

JAEA Reports

None

; ; ; ; *

PNC TN8410 91-237, 31 Pages, 1991/09

PNC-TN8410-91-237.pdf:0.57MB

None

Journal Articles

Dissolution of plutonium dioxide by electrolytic method, 1

Sakurai, Satoshi; Tachimori, Shoichi; Akatsu, Jokun; Kimura, Takaumi; Yoshida, Zenko; ; Yamashita, Toshiyuki; Ouchi, Kinji

Nihon Genshiryoku Gakkai-Shi, 31(11), p.1243 - 1250, 1989/11

 Times Cited Count:3 Percentile:41.84(Nuclear Science & Technology)

no abstracts in English

Journal Articles

The Effect of rare earths on thermal conductivity of uranium,plutonium and their mixed oxide fuels

; ;

J.Less-Common Met., 121, p.631 - 636, 1986/00

 Times Cited Count:13 Percentile:80.28(Chemistry, Physical)

no abstracts in English

Journal Articles

Removal of americium by its evaporation during carbo-thermic reduction of plutonium dioxide

; ;

Journal of Nuclear Science and Technology, 22(4), p.329 - 330, 1985/00

 Times Cited Count:3 Percentile:53.49(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Carbothermic synthesis of plutonium mononitride from the dioxide

; ;

Journal of Nuclear Materials, 115, p.331 - 333, 1983/00

 Times Cited Count:5 Percentile:85.28(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Mechanism of carbothermic reduction of(U,Pu)O$$_{2}$$ to(U,Pu)C

; ; ;

Journal of Nuclear Science and Technology, 20(10), p.874 - 876, 1983/00

 Times Cited Count:1 Percentile:27.09(Nuclear Science & Technology)

no abstracts in English

JAEA Reports

None

; *; Komatsu, Junji*; Kawata, Tomio*

PNC TN243 81-03, 24 Pages, 1981/10

PNC-TN243-81-03.pdf:0.6MB

None

JAEA Reports

KENO-IV Code Benchmark Calculation,6; Plutonium Fuel in Various Shape

; ; *

JAERI-M 9201, 51 Pages, 1980/11

JAERI-M-9201.pdf:2.78MB

no abstracts in English

Journal Articles

Electrical conductivity anomaly in near-stoichiometric plutonium dioxide

*; *; ; ; ; Tagawa, Hiroaki

Journal of Nuclear Materials, 95, p.181 - 184, 1980/00

 Times Cited Count:13 Percentile:77.12(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Behavior of ruthenium in fluoride-volatility process, 1; Fluorination of PuO$$_{2}$$-RuO$$_{2}$$ mixture and recovery of plutonium by thermal decomposition

; ;

Journal of Nuclear Science and Technology, 11(2), p.74 - 76, 1974/02

 Times Cited Count:3

no abstracts in English

14 (Records 1-14 displayed on this page)
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